Targeting the carbon graphite sealing materials and sealing technology for aero-engine, the typical application scenarios, development history, failure modes, research status at home and abroad, as well as the service performance requirements of carbon-graphite sealing materials in aero-engine sealing systems were described in detail. The advantages and disadvantages of its different preparation processes were emphasized, and suggestions were made for its future development direction. The results showed that carbon graphite sealing materials are widely used in aero engines. The physical properties of carbon graphite sealing materials independently developed in China were very close to those abroad, and some indicators were even better. They basically met the material selection requirements for China’s new generation of high-performance aero-engine, and important models achieved independent controllability. However, the batch stability, processability, homogeneity, high temperature oxidation resistance, film formation, friction factor, wear rate and service life of some domestic carbon graphite sealing materials still had a certain gap with foreign original carbon graphite sealing materials for aircraft engines in the process of long-term service, mainly due to the failure of domestic carbon graphite sealing materials to achieve the effective construction of structure-function integration.